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It takes about 3/4 of a tank, but the Big Daddy won't be able to move as you shoot and kill him. Try using Electric Gel in the Chemical Thrower. Here's another easy method to kill Big Daddies easily.
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This method usually results in a one-hit kill and is especially useful against higher-level Splicers.
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Set a key binding to the following codes (for example, "F10=fly"). Use a text editor to edit the "defuser.ini" file in the game directory. This procedure involves editing a game file create a backup copy of the file before proceeding. Search for the section called and find the unbound key that you want to use and bind it to the command "Exec upgrades.txt" (F7=Exec upgrades.txt). In “X:Documents and SettingsApplication DataBioshock” (XP) or “X:UsersAppDataRoamingBioShock” (Vista), open the file named “User.ini” - you need to enable viewing of hidden files and folders.